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Intense-field modulation of NO2 multiphoton dissociation dynamics

Lookup NU author(s): Dr Gareth Roberts

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Abstract

The dissociation of NO2 under strong-field conditions by femtosecond two-color fluorescence depletion spectroscopy was reported. The dissociation dynamics were interpreted in terms of nuclear motions over light-induced potentials formed by coupling of NO2 valence and Rydberg states to the applied field. It was found that generation of nā€² = 0 and 1 NO A2āˆ‘+ results in different fluorescence modulation patterns. The time required for three-photon dissociation of NO 2 to give NO A2āˆ‘+ and O3P at Terawatt intensities was also observed.

Publication metadata

Author(s): Schmidt TW, Lopez-Martens RB, Roberts G

Publication type: Article

Publication status: Published

Journal: Journal of Chemical Physics

Year: 2004

Volume: 121

Issue: 9

Pages: 4133-4142

ISSN (print): 0021-9606

ISSN (electronic): 1520-9032

Publisher: American Institute of Physics

URL: http://dx.doi.org/10.1063/1.1775768

DOI: 10.1063/1.1775768

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